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Room-temperature aqueous monolithic in situ integration enables quasi-single-crystalline PbS photodetectors on ROICs with carrier density ~2 × 10^15 cm^-3 and mobility 124 cm^2 V^-1 s^-1.
Chalcogenide Semiconductor Thin Films
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Bismuth sulfide (Bi2S3) exhibits a pseudo-direct bandgap, with a lower-energy indirect transition paired with a direct transition a few kBT above, enabling delayed bimolecular electron-hole recombination.
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Molecular regulation of metal-organic coordination suppresses cross-linked precursor networks, enabling blade-coated kesterite Cu2ZnSn(S,Se)4 films over 10 cm2 with 13.0% module efficiency.
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