Radical-based heteroatom homolytic substitution enables efficient synthesis of sterically congested dialkyl ethers, surpassing classical methods with a broad scope of substitution patterns.
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Pyridoxal 5'-phosphate (PLP) acts as a photoenzymatic cofactor enabling asymmetric radical-radical cross-couplings, expanding enzymatic bond formation capabilities.
Vicinal disubstitution of alkyl C-X synthons is achieved via alkene radical cation generation, enabling 1,2-difunctionalization with broad nucleophile compatibility.
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